Bigglypuff
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Bigglypuff is a giant Jigglypuff who appeared in The Ancient Puzzle of Pokémopolis. It has strange markings all over it and has a much deeper voice than a regular Jigglypuff. When it sings, it uses a bell as a microphone, and a paintbrush as a marker.
When the giant Gengar and Alakazam were fighting, it threatened to destroy the world. Jigglypuff attempted to Sing its song, but the two giant Pokémon were not affected by it. Gengar knocked Alakazam into Jigglypuff, sending it flying. Although it failed to make the giants fall asleep, Jigglypuff did activate an ancient artifact, which released a giant Jigglypuff. It started singing, and unlike its normal-sized counterpart, put everyone to sleep. However, like it's counterpart, when it saw everyone sleeping, it drew on their faces.
Upon awakening, Ash and the others noticed all the giant Pokémon had vanished, leaving only the artifacts they came out of.